Beleaguered Pochettino is under pressure after Spurs were humiliated 7-2 at home by Bayern Munich in the Champions League on Tuesday night.
It means that the Argentine has become the new 6/4 favourite to be the next top-flight manager to leave his post - having been 12/1 beforehand.
Meanwhile, former Chelsea and Manchester United boss Mourinho has been installed as the favourite to be the next Spurs manager at 3/1.
He is ahead of the former Juventus manager Massimiliano Allegri at 5/1 and the current Bournemouth boss Eddie Howe at 6/1, according to SportNation.bet.
Mourinho has not taken another managerial job since then, instead working as a television pundit.
Both Mourinho and Allegri have the pedigree to end Spurs' long wait for a piece of silverware. Their last taste of success was winning the League Cup in 2008 though they did reach the Champions League final last season.
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